KIP-Veröffentlichungen

Jahr 2017
Autor(en) Anton Kuzyk, Maximilian J. Urban, Andrea Idili, Francesco Ricci and Na Liu
Titel Selective control of reconfigurable chiral plasmonic metamolecules
KIP-Nummer HD-KIP 17-77
KIP-Gruppe(n) F28
Dokumentart Paper
Keywords (angezeigt) DNA nanotechnology, Self assembly, active plasmonics, Circular Dichroism, enantioselectivity
Quelle Science Advances 3 (2017) 4, e1602803
doi 10.1126/sciadv.1602803
Abstract (en)

Selective configuration control of plasmonic nanostructures using either top-down or bottom-up approaches has remained challenging in the field of active plasmonics. We demonstrate the realization of DNA-assembled reconfigurable plasmonic metamolecules, which can respond to a wide range of pH changes in a programmable manner. This programmability allows for selective reconfiguration of different plasmonic metamolecule species coexisting in solution through simple pH tuning. This approach enables discrimination of chiral plasmonic quasi-enantiomers and arbitrary tuning of chiroptical effects with unprecedented degrees of freedom. Our work outlines a new blueprint for implementation of advanced active plasmonic systems, in which individual structural species can be programmed to perform multiple tasks and functions in response to independent external stimuli.

bibtex
@article{NaLiu2017,
  author   = {Anton Kuzyk, Maximilian J. Urban, Andrea Idili, Francesco Ricci and Na Liu},
  title    = {Selective control of reconfigurable chiral plasmonic metamolecules},
  journal  = {Science Advances},
  year     = {2017},
  volume   = {3},
  number   = {4},
  pages    = {e1602803},
  month    = {April},
  doi      = {10.1126/sciadv.1602803},
  url      = {http://advances.sciencemag.org/content/3/4/e1602803}
}
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